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Hester, Gavin; DeLazzer, T N; Yahne, D R; Sarkis, C L; Zhao, H D; Rivera, J A; Calder, S; Ross, K A (, Journal of Physics: Condensed Matter)
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Daum, M. J.; Ramanathan, A.; Kolesnikov, A. I.; Calder, S.; Mourigal, M.; La Pierre, H. S. (, Physical Review B)null (Ed.)
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Reig-i-Plessis, D.; Johnson, T. A.; Lu, K.; Chen, Q.; Ruff, J. P.; Upton, M. H.; Williams, T. J.; Calder, S.; Zhou, H. D.; Clancy, J. P.; et al (, Physical Review Materials)null (Ed.)
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Sarte, P. M.; Cruz-Kan, K.; Ortiz, B. R.; Hong, K. H.; Bordelon, M. M.; Reig-i-Plessis, D.; Lee, M.; Choi, E. S.; Stone, M. B.; Calder, S.; et al (, npj Quantum Materials)Abstract The magnetic ground state of the pyrochlore Yb 2 GaSbO 7 has not been established. The persistent spin fluctuations observed by muon spin-relaxation measurements at low temperatures have not been adequately explained for this material using existing theories for quantum magnetism. Here we report on the synthesis and characterisation of Yb 2 GaSbO 7 to revisit the nature of the magnetic ground state. Through DC and AC magnetic susceptibility, heat capacity, and neutron scattering experiments, we observe evidence for a dynamical ground state that makes Yb 2 GaSbO 7 a promising candidate for disorder-induced spin-liquid or spin-singlet behaviour. This state is quite fragile, being tuned to a splayed ferromagnet in a modest magnetic field μ 0 H c ~ 1.5 T.more » « less
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